#METABOLOMICS WORKBENCH flazando_20221111_050439 DATATRACK_ID:3565 STUDY_ID:ST002401 ANALYSIS_ID:AN003912 VERSION 1 CREATED_ON 02-08-2024 #PROJECT PR:PROJECT_TITLE Human primary astrocytes finger- and footprinting metabolomics indicate PR:PROJECT_TITLE biochemical alterations under ayahuasca treatment PR:PROJECT_TYPE Untargetmetabomics- hilic PR:PROJECT_SUMMARY Ayahuasca (Aya) is a psychotropic Amazonian beverage formulated from the PR:PROJECT_SUMMARY combination of the Banisteriopsis caapi vine and the Psychotria viridis leaves PR:PROJECT_SUMMARY in a water decoction. Aya is legally used in Latin American countries and used PR:PROJECT_SUMMARY in Brazil for religious, cultural, and therapeutic purposes. Its properties PR:PROJECT_SUMMARY constitute a bio-psycho-social-spiritual model involving effects from PR:PROJECT_SUMMARY ß-carboline-derived alkaloids, present in the vine, and N,N-dimethyltryptamine PR:PROJECT_SUMMARY (DMT), a tryptamine-derived alkaloid present in the leaves, which act together PR:PROJECT_SUMMARY in the central nervous system (CNS). Few technical-scientific studies have been PR:PROJECT_SUMMARY conducted to understand the effects of this brew in the metabolism. Therefore, PR:PROJECT_SUMMARY this work aims to investigate an in vitro primary astrocyte lineage model by PR:PROJECT_SUMMARY untargeted metabolomics evaluations of two cellular subfractions: secretome and PR:PROJECT_SUMMARY intracellular content after Aya treatment, where DMT and other ß-carbolines PR:PROJECT_SUMMARY were previously quantified. Metabolomics analysis was performed by UHPLC-MS/MS, PR:PROJECT_SUMMARY followed by MS-Dial data processing and statistical analysis to identify PR:PROJECT_SUMMARY metabolites and biochemical alterations related to Aya treatment. Aya doses were PR:PROJECT_SUMMARY applied to the cell cultures considering DMT concentrations of 1, 10 and 20 µM, PR:PROJECT_SUMMARY which are in agreement with non-toxic and toxic DMT threshold assays in primary PR:PROJECT_SUMMARY human astrocyte cells viability. PR:INSTITUTE University of Campinas PR:DEPARTMENT Analytical Chemistry Department PR:LABORATORY Laboratory of Bioanalytics and Integrated Omics (LABIOmics) PR:LAST_NAME Zandonadi PR:FIRST_NAME Flavia PR:ADDRESS Rua Josué de Castro, s/n - Cidade Universitária, Campinas - SP, 13083-970 PR:EMAIL flazando@unicamp.br PR:PHONE +551935213038 PR:FUNDING_SOURCE Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES) [grant PR:FUNDING_SOURCE number: 88882.305841/2018-01]. Fundação de Amparo à Pesquisa do Estado de PR:FUNDING_SOURCE São Paulo - FAPESP [grant number: 2018/01525-3] and INCT de Bioanalítica PR:FUNDING_SOURCE [grant numbers: FAPESP 2014/50867-3 and CNPq 465389/2014-7] PR:DOI http://dx.doi.org/10.21228/M8QT3T #STUDY ST:STUDY_TITLE Human primary astrocytes finger- and footprinting metabolomics indicate ST:STUDY_TITLE biochemical alterations under ayahuasca treatment ST:STUDY_SUMMARY Ayahuasca (Aya) is a psychotropic Amazonian beverage formulated from the ST:STUDY_SUMMARY combination of the Banisteriopsis caapi vine and the Psychotria viridis leaves ST:STUDY_SUMMARY in a water decoction. Aya is legally used in Latin American countries and used ST:STUDY_SUMMARY in Brazil for religious, cultural, and therapeutic purposes. Its properties ST:STUDY_SUMMARY constitute a bio-psycho-social-spiritual model involving effects from ST:STUDY_SUMMARY β-carboline-derived alkaloids, present in the vine, and N,N-dimethyltryptamine ST:STUDY_SUMMARY (DMT), a tryptamine-derived alkaloid present in the leaves, which act together ST:STUDY_SUMMARY in the central nervous system (CNS). Few technical-scientific studies have been ST:STUDY_SUMMARY conducted to understand the effects of this brew in the metabolism. Therefore, ST:STUDY_SUMMARY this work aims to investigate an in vitro primary astrocyte lineage model by ST:STUDY_SUMMARY untargeted metabolomics evaluations of two cellular subfractions: secretome and ST:STUDY_SUMMARY intracellular content after Aya treatment, where DMT and other β-carbolines ST:STUDY_SUMMARY were previously quantified. Metabolomics analysis was performed by UHPLC-MS/MS, ST:STUDY_SUMMARY followed by MS-Dial data processing and statistical analysis to identify ST:STUDY_SUMMARY metabolites and biochemical alterations related to Aya treatment. Aya doses were ST:STUDY_SUMMARY applied to the cell cultures considering DMT concentrations of 1, 10 and 20 µM, ST:STUDY_SUMMARY which are in agreement with non-toxic and toxic DMT threshold assays in primary ST:STUDY_SUMMARY human astrocyte cells viability ST:INSTITUTE University of Campinas ST:LAST_NAME Zandonadi ST:FIRST_NAME Flavia ST:ADDRESS Rua Josué de Castro, s/n - Cidade Universitária, Campinas - SP, 13083-970 ST:EMAIL flazando@unicamp.br ST:PHONE +551935213038 ST:SUBMIT_DATE 2022-11-11 #SUBJECT SU:SUBJECT_TYPE Cultured cells SU:SUBJECT_SPECIES Homo sapiens SU:TAXONOMY_ID 9606 SU:AGE_OR_AGE_RANGE 14-36 SU:CELL_PASSAGE_NUMBER 4 #SUBJECT_SAMPLE_FACTORS: SUBJECT(optional)[tab]SAMPLE[tab]FACTORS(NAME:VALUE pairs separated by |)[tab]Additional sample data SUBJECT_SAMPLE_FACTORS Intracellular E1_Aya10_intra_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E1_Aya10_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya10_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E1_Aya10_sec_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E1_Aya10_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya10_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E2_Aya10_intra_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E2_Aya10_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya10_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E2_Aya10_sec_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E2_Aya10_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya10_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E3_Aya10_intra_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E3_Aya10_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya10_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E3_Aya10_sec_HILIC_POS Treatment:Aya 10 µM DTT-based RAW_FILE_NAME=E3_Aya10_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya10_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E1_Aya1_intra_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E1_Aya1_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya1_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E1_Aya1_sec_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E1_Aya1_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya1_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E2_Aya1_intra_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E2_Aya1_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya1_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E2_Aya1_sec_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E2_Aya1_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya1_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E3_Aya1_intra_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E3_Aya1_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya1_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E3_Aya1_sec_HILIC_POS Treatment:Aya 1 µM DTT-based RAW_FILE_NAME=E3_Aya1_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya1_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E1_Aya20_intra_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E1_Aya20_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya20_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E1_Aya20_sec_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E1_Aya20_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya20_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E2_Aya20_intra_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E2_Aya20_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya20_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E2_Aya20_sec_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E2_Aya20_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya20_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E3_Aya20_intra_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E3_Aya20_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya20_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E3_Aya20_sec_HILIC_POS Treatment:Aya 20 µM DTT-based RAW_FILE_NAME=E3_Aya20_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya20_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E1_AyaDMSO_intra_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E1_AyaDMSO_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E1_AyaDMSO_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E1_AyaDMSO_sec_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E1_AyaDMSO_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E1_AyaDMSO_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E2_AyaDMSO_intra_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E2_AyaDMSO_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E2_AyaDMSO_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E2_AyaDMSO_sec_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E2_AyaDMSO_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E2_AyaDMSO_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E3_AyaDMSO_intra_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E3_AyaDMSO_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E3_AyaDMSO_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E3_AyaDMSO_sec_HILIC_POS Treatment:Negative Control RAW_FILE_NAME=E3_AyaDMSO_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E3_AyaDMSO_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E1_Aya0_intra_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E1_Aya0_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya0_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E1_Aya0_sec_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E1_Aya0_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E1_Aya0_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E2_Aya0_intra_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E2_Aya0_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya0_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E2_Aya0_sec_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E2_Aya0_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E2_Aya0_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular E3_Aya0_intra_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E3_Aya0_intra_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya0_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) E3_Aya0_sec_HILIC_POS Treatment:Positive Control RAW_FILE_NAME=E3_Aya0_sec_HILIC_NEG.mzML; RAW_FILE_NAME=E3_Aya0_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular QC_10_intra_HILIC_POS Treatment:Quality Control RAW_FILE_NAME=QC_10_intra_HILIC_NEG.mzML; RAW_FILE_NAME=QC_10_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular QC_1_intra_HILIC_POS Treatment:Quality Control RAW_FILE_NAME=QC_1_intra_HILIC_NEG.mzML; RAW_FILE_NAME=QC_1_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Intracellular QC_20_intra_HILIC_POS Treatment:Quality Control RAW_FILE_NAME=QC_20_intra_HILIC_NEG.mzML; RAW_FILE_NAME=QC_20_intra_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) QC_10_sec_HILIC_POS Treatment:Quality Control Aya 10 µM DTT-based group RAW_FILE_NAME=QC_10_sec_HILIC_NEG.mzML; RAW_FILE_NAME=QC_10_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) QC_1_sec_HILIC_POS Treatment:Quality Control Aya 1 µM DTT-based group RAW_FILE_NAME=QC_1_sec_HILIC_NEG.mzML; RAW_FILE_NAME=QC_1_sec_HILIC_POS.mzML SUBJECT_SAMPLE_FACTORS Secretome (Extracellular) QC_20_sec_HILIC_POS Treatment:Quality Control Aya 20 µM DTT-based group RAW_FILE_NAME=QC_20_sec_HILIC_NEG.mzML; RAW_FILE_NAME=QC_20_sec_HILIC_POS.mzML #COLLECTION CO:COLLECTION_SUMMARY The astrocyte cells were obtained in collaboration with the Nervous Regeneration CO:COLLECTION_SUMMARY Laboratory (Prof. Dr. Alexandre Oliveira), Institute of Biology, UNICAMP, CO:COLLECTION_SUMMARY Brazil. CO:SAMPLE_TYPE Astrocytes CO:STORAGE_CONDITIONS -80℃ #TREATMENT TR:TREATMENT_SUMMARY Aya doses were applied to the cell cultures considering DMT concentrations of 1, TR:TREATMENT_SUMMARY 10 and 20 µM, which are in agreement with non-toxic and toxic DMT threshold TR:TREATMENT_SUMMARY assays in primary human astrocyte cells viability.secretome (extracellular TR:TREATMENT_SUMMARY fraction) were collected, centrifuged under 500 x g at room temperature (about TR:TREATMENT_SUMMARY 27 ºC) for 5 min, stored and conditioned at -80 °C until the time of TR:TREATMENT_SUMMARY metabolomics sample preparation. In parallel, to obtain the content of TR:TREATMENT_SUMMARY intracellular metabolites, cell monolayers were washed three times with 5 mL of TR:TREATMENT_SUMMARY ice-cold PBS to remove any excess of secretome. Subsequently, a mechanical TR:TREATMENT_SUMMARY detachment was performed for removal, followed by chemical rupture of the cell TR:TREATMENT_SUMMARY wall in 1.2 mL of ice-cold 80 % (v/v) methanol in PBS solution, to obtain an TR:TREATMENT_SUMMARY intracellular metabolite suspension. The intracellular fractions, in methanol TR:TREATMENT_SUMMARY solution, were stored and conditioned at -80 °C. #SAMPLEPREP SP:SAMPLEPREP_SUMMARY For metabolomics analysis, after being defrosted, the secretome samples volumes SP:SAMPLEPREP_SUMMARY were reduced to 500 μL by centrifugation in an Amicon® Ultra-2 mL (Millipore) SP:SAMPLEPREP_SUMMARY filter, according to the manufacturer specifications. Then, quality control (QC) SP:SAMPLEPREP_SUMMARY samples were prepared previously to the protein precipitation. Ice-cold 80 % SP:SAMPLEPREP_SUMMARY (v/v) methanol was added to the concentrated secretome, kept at -80 °C, as well SP:SAMPLEPREP_SUMMARY as the intracellular fraction, for the protein precipitation step for 24 h. SP:SAMPLEPREP_SUMMARY After that period of time, all samples (extra and intracellular metabolite SP:SAMPLEPREP_SUMMARY suspensions) were centrifuged at 16,000 x g at 4 °C for 15 min, the SP:SAMPLEPREP_SUMMARY supernatants filtered in a 0.22 μm syringe filter, and dried in a vacuum SP:SAMPLEPREP_SUMMARY concentrator. For each cellular fraction, 12 samples were included in the SP:SAMPLEPREP_SUMMARY analysis, where three (3) experimental samples for each group were identified as SP:SAMPLEPREP_SUMMARY Aya0, Aya1, Aya10, or Aya20, corresponding to DMT doses in µmol L-1, and five SP:SAMPLEPREP_SUMMARY (5) for QC samples, being four (4) QC related to dose-treatments and one (1) to SP:SAMPLEPREP_SUMMARY all treatment groups. SP:SAMPLEPREP_PROTOCOL_FILENAME Samplepreparation_zandonadi22.pdf SP:PROCESSING_STORAGE_CONDITIONS -80℃ SP:EXTRACT_STORAGE On ice #CHROMATOGRAPHY CH:CHROMATOGRAPHY_SUMMARY Acquity BEH Amide column (2.1 mm x 150 mm, 1.7 μm particle size, Waters Corp.) CH:CHROMATOGRAPHY_SUMMARY for hydrophilic interaction liquid chromatography (HILIC). The sample injection CH:CHROMATOGRAPHY_SUMMARY volume was set to 5 μL and the column temperature was kept at 45 °C. CH:CHROMATOGRAPHY_SUMMARY Separation was performed at a 0.4 mL min-1 flow rate under a gradient program in CH:CHROMATOGRAPHY_SUMMARY which the mobile phases consisted of: (A) 10 mmol L-1 ammonium acetate in ACN: CH:CHROMATOGRAPHY_SUMMARY water (95: 5) and (B) 10 mmol L-1 ammonium acetate in ACN: water (50:50). The CH:CHROMATOGRAPHY_SUMMARY gradient started with 1% B for 1 min, increasing to 100% B for 9 min and CH:CHROMATOGRAPHY_SUMMARY subsequently returning to 1% B in 0.1 min. Over the next 3.9 min, the column was CH:CHROMATOGRAPHY_SUMMARY re-equilibrated before the next injection. Total execution time was 14 min. CH:METHODS_FILENAME UntargetHilicmethodXEVO_zandonadi22.pdf CH:INSTRUMENT_NAME Waters Acquity CH:COLUMN_NAME Waters Acquity BEH HILIC (150 x 2.1mm, 1.7um) CH:COLUMN_TEMPERATURE 45 °C CH:FLOW_GRADIENT 1 % B for 1 min, increasing to 100% B for 9 min and subsequently returning to 1 CH:FLOW_GRADIENT % B in 0.1 min. Over the next 3.9 min, the column was re-equilibrated before the CH:FLOW_GRADIENT next injection. Total execution time was 14 min CH:FLOW_RATE 0.4 mL min-1 CH:SOLVENT_A 95% acetonitrile/5% water; 10 mM ammonium acetate CH:SOLVENT_B 50% acetonitrile/50% water; 10mM ammonium acetate CH:CHROMATOGRAPHY_TYPE HILIC #ANALYSIS AN:ANALYSIS_TYPE MS #MS MS:INSTRUMENT_NAME Waters Xevo-G2-XS MS:INSTRUMENT_TYPE QTOF MS:MS_TYPE ESI MS:MS_COMMENTS Detection was performed using a XEVO-G2XS quadrupole time-of-flight (QTOF) mass MS:MS_COMMENTS spectrometer (Waters Corp., Manchester, UK) equipped with an electrospray MS:MS_COMMENTS ionization (ESI) source. Data were collected in both positive and negative MS:MS_COMMENTS ionization modes, separately. The acquisition was performed using MS:MS_COMMENTS data-independent analysis (MSE), with the following parameters: capillary MS:MS_COMMENTS voltage +3.5 kV (positive mode) and -2.5 kV (negative mode), sample cone voltage MS:MS_COMMENTS at 40 kV, source temperature at 140 °C, desolvation temperature of 550 °C, MS:MS_COMMENTS desolvation gas flow of 900 L h−1, and cone gas flow of 10 L h−1 (positive MS:MS_COMMENTS mode) or 50 L h−1 (negative mode). MS data were acquired in the centroid mode MS:MS_COMMENTS from m/z range of 50–1200 Da, using the acquisition rate of 0.5 s per scan. MS:MS_COMMENTS The MSE analysis was operated at 20 V for low collision energy and 50 V for high MS:MS_COMMENTS collision energy. During MS analysis, a leucine enkephalin (Waters®, molecular MS:MS_COMMENTS mass = 555.62; 200 pg μL-1 in 1:1 ACN: H2O) was continuously infused into MS at MS:MS_COMMENTS a flow rate of 30 µL min-1 and the ions [M-H]- = 554.26 and [M+H]+ = 556.27 MS:MS_COMMENTS were used as lock mass for accurate mass measurement. Data acquisition was MS:MS_COMMENTS controlled by MassLynx V4.2 (Waters®). Calibration was performed prior to MS:MS_COMMENTS sample analysis via infusion of 0.5 mmol L-1 sodium formate solution, which was MS:MS_COMMENTS used for calibration procedures, both in positive and negative mode analysis. MS:MS_COMMENTS Samples were randomly analyzed and QC samples composed of pooled samples after MS:MS_COMMENTS resuspension were injected every 8 injections. Data processing and metabolite MS:MS_COMMENTS identification. All MSE datasets were converted from the vendor-specific file MS:MS_COMMENTS format (.raw) into the Analysis Base File format (.abf) using the freely MS:MS_COMMENTS available Reifycs ABF converter MS:MS_COMMENTS (https://www.reifycs.com/AbfConverter/index.html). After conversion, the MS-DIAL MS:MS_COMMENTS software (version 5.0) was used for feature detection, spectral deconvolution, MS:MS_COMMENTS peak identification, and alignment between samples. MassBank databases were used MS:MS_COMMENTS for identification from MS-DIAL metabolomics MSP spectral kit containing ESI-MS MS:MS_COMMENTS and MS/MS (positive; 8,068 and negative; 4,782 compounds). MS:MS_COMMENTS (http://prime.psc.riken.jp/compms/msdial/main.html). The parameters for MS-DIAL MS:MS_COMMENTS were optimized based on their based on developer instructions. The UHPLC-MS raw MS:MS_COMMENTS data were processed with MS-DIAL version 4.8 [30]. Automatic feature detection MS:MS_COMMENTS was performed between 0.3 and 13 min for mass signal extraction between 100 and MS:MS_COMMENTS 1500 Da in positive and negative modes. MS1 and MS2 tolerance were set to 0.01 MS:MS_COMMENTS and 0.4 Da, respectively, in profile mode. For identification, it was used the MS:MS_COMMENTS default of accurate mass tolerance 0.01 Da for MS1 and 0.05 Da for MS2, and MS:MS_COMMENTS identification score cut off 80 %. For the potential adducts, [M+H]+, [M+Na]+, MS:MS_COMMENTS [M+K]+, [M+NH4]+, [2M+H]+, [M+2H]2+, [M+2Na]2+, [M+2K]2+, [M+H+Na]2+, [M+H+K]2+, MS:MS_COMMENTS [M+H+NH4]2+, [M+2Na-H]+, [M+2K-H]+, [M+H-H2O]+, and [M+H-2H2O]+ were considered MS:MS_COMMENTS for positively charged adducts, while [M-H]-, [M+Cl]-, [M-H-H2O]-, [2M-H]-, MS:MS_COMMENTS [M-2H]2-, [M+Na-2H]-, [M+K-2H]-, and [M+FA-H]- were considered for negatively MS:MS_COMMENTS charged. To generate matrix files for downstream statistical analysis, the MS:MS_COMMENTS aligned results were exported by selecting the area raw data matrix, that were MS:MS_COMMENTS restructured by applying a manual exclusion filter for unknown metabolites, and MS:MS_COMMENTS the negative and positive files were combined for statistical analysis in MS:MS_COMMENTS MetaboAnalyst 5.0 [31]. MS:ION_MODE POSITIVE MS:MS_RESULTS_FILE ST002401_AN003912_Results.txt UNITS:TIC Has m/z:Yes Has RT:Yes RT units:Minutes #END